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From my own experience, it seems that the tentacle makes all procs crit. Or at least that's what it looks like when I use it after letting SS stack to 100% crit.
That's been my experience as well.
This is inaccurate because the Sharpshooter 100% crit buff won't actually go away until one second after the first crit has landed.
In these cases, it's actually fairly trivial to get 3 or 4 NT balls with guaranteed crit fire.
This is simple to test, and my testing indicates that the crit RNG is calculated on each individual proc. You can turn on white damage numbers in your options, which will stand out against your yellow damage crits.
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